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Technologies for pollutant removal and resource recovery from blackwater: a review

《环境科学与工程前沿（英文）》 2023年第17卷第7期 doi: 10.1007/s11783-023-1683-3

摘要：

● Blackwater is the main source of organics and nutrients in domestic wastewater.

关键词： Blackwater Water-flushing toilet Sanitation Nutrient recovery Water reuse Sustainable development

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China Launched the First Wastewater Resource Recovery Factory in Yixing

《环境科学与工程前沿（英文）》 2022年第16卷第1期 doi: 10.1007/s11783-021-1496-1

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“NEW” resource recovery from wastewater using bioelectrochemical systems: Moving forward with functions

Akshay Jain, Zhen He

《环境科学与工程前沿（英文）》 2018年第12卷第4期 doi: 10.1007/s11783-018-1052-9

摘要：

Resource recovery from wastewater is a key function of bioelectrochemical systems.

NEW resources to recover include Nutrient, Energy, and Water.

Identifying proper application niches can guide BES research and development.

More efforts should be invested to the application of recovered resources.

A mindset for energy performance and system scaling is critically important.

关键词： Bioelectrochemical systems Resource recovery Wastewater treatment Energy Nutrients

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Bio-based Technologies for Resource Recovery

Aijie Wang, David Stuckey

《环境科学与工程前沿（英文）》 2018年第12卷第4期 doi: 10.1007/s11783-018-1079-y

摘要：

关键词： valign= top class= J_zhaiyao

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LivestockWaste 2016-International Conference on Recent Advances in Pollution Control and ResourceRecovery for the Livestock Sector

Xinmin Zhan, Liwen Xiao

《环境科学与工程前沿（英文）》 2017年第11卷第3期 doi: 10.1007/s11783-017-0958-y

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Sea salt bittern-driven forward osmosis for nutrient recovery from black water: A dual waste-to-resource

Wenchao Xue, May Zaw, Xiaochan An, Yunxia Hu, Allan Sriratana Tabucanon

《环境科学与工程前沿（英文）》 2020年第14卷第2期 doi: 10.1007/s11783-019-1211-7

摘要： • A dual “waste-to-resource” application of FO was proposed. • Performance of sea salt bittern as an economic FO draw solution was evaluated. • High quality struvite recovery from black water using FO was demonstrated. • Feed pH is a key factor to control the form of recovered phosphorous. A dual “waste-to-resource” innovation in nutrient enrichment and recovery from domestic black water using a sea salt bittern (SSB)-driven forward osmosis (FO) process is proposed and demonstrated. The performance of SSB as a “waste-to-resource” draw solution for FO was first evaluated. A synthetic SSB-driven FO provided a water flux of 25.67±3.36 L/m2⋅h, which was 1.5‒1.7 times compared with synthetic seawater, 1 M NaCl, and 1 M MgCl2. Slightly compromised performance regarding reverse solute selectivity was observed. In compensation, the enhanced reverse diffusion of Mg2+ suggested superior potential in terms of recovering nutrients in the form of struvite precipitation. The nutrient enrichment was performed using both the pre-filtered influent and effluent of a domestic septic tank. Over 80% of phosphate-P recovery was achieved from both low- and high-strength black water at a feed volume reduction up to 80%‒90%. With an elevated feed pH (~9), approximately 60%‒85% enriched phosphate-P was able to be recovered in the form of precipitated stuvite. Whereas the enrichment performance of total Kjeldahl nitrogen (TKN) largely differed depending on the strength of black water. Improved concentration factor (i.e., 3-folds) and retention (>60%) of TKN was obtained in the high-nutrient-strength black water at a feed volume reduction of 80%, in comparison with a weak TKN enrichment observed in low-strength black water. The results suggested a good potential for nutrient recovery based on this dual “waste-to-resource” FO system with proper management of membrane cleaning.

关键词： Forward osmosis Sea salt bittern Black water Nutrient recovery pH

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我国城镇污泥安全处置与资源化研究

戴晓虎,侯立安,章林伟,张林,杨东海

《中国工程科学》 2022年第24卷第5期页码 145-153 doi: 10.15302/J-SSCAE-2022.05.017

摘要：

污泥作为污水处理的过程产物，具有“污染”“资源”双重属性，对其开展妥善处置是污水处理减污降碳的重要任务。虽然我国污泥处理经历了“重水轻泥”向“泥水并重”的转变，技术与标准体系发展迅速，但在生态文明建设，碳达峰、碳中和目标的背景下，污泥处理处置仍存在亟待突破的短板弱项。本文梳理了城镇污泥产量和泥质特征、处理处置技术、政策标准体系的发展现状，凝练了污泥处理处置在管理体系、技术标准、路线选择等方面存在的突出问题；结合我国所处的发展阶段和国际发展趋势，提出了“绿色低碳、资源循环、环境友好、因地制宜”的发展理念以及相应的重点举措。研究建议，加强顶层设计，统筹设施规划布局，因地制宜选择处理处置路线；健全污泥处理处置的标准体系，完善价格补贴机制，强化责任分工与监管机制；补短板、强弱项，提升全链条集成水平，形成可推广的技术模式；面向未来实施前沿技术攻关，推动污泥处理处置与资源化技术装备创新升级。

关键词：污水厂污泥；污泥处理；污染控制；资源回收；减污降碳

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Power-to-chemicals: sustainable liquefaction of food waste with plasma-electrolysis

《化学科学与工程前沿（英文）》 2023年第17卷第5期页码 594-605 doi: 10.1007/s11705-022-2255-y

摘要： The increasing amount of food waste from various industrial, agricultural, and household sources is an environmental burden if managed inappropriately. Numerous waste management approaches have been developed for the disposal of food waste, but still suffer from either high cost, production of toxic by-products, or secondary environmental pollutions. Herein, we report a new and sustainable plasma electrolysis biorefinery route for the rapid and efficient liquefaction of food waste. During the plasma electrolysis process, only the solvent is added to liquefy the waste, and anions in the waste can contribute to catalyzing the biowaste conversion. While liquefying the waste, the highly reactive species produced in the plasma electrolysis process can efficiently reduce the content of O, N, and Cl in the liquefied products and oxidize most of the metals into solid residues. Especially, the removal rate of Na and K elements was greater than 81%, which is significantly higher than using the traditional oil bath liquefaction, resulting in a relatively high-quality biocrude oil with a high heating value of 25.86 MJ·kg^–1. Overall, this proposed strategy may provide a new sustainable and eco-friendly avenue for the power-to-chemicals valorization of food waste under benign conditions.

关键词： plasma electrolysis food waste liquefaction resource recovery

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Nanoscale Zero-Valent Iron (nZVI) for Heavy Metal Wastewater Treatment: A Perspective

Shaolin Li,Lei Li,Weixian Zhang,

《工程（英文）》 doi: 10.1016/j.eng.2023.08.012

摘要： Industries such as non-ferrous metal smelting discharge billions of gallons of highly toxic heavy metal wastewater (HMW) worldwide annually, posing a severe challenge to conventional wastewater treatment plants and harming the environment. HMW is traditionally treated via chemical precipitation using lime, caustic, or sulfide, but the effluents do not meet the increasingly stringent discharge standards. This issue has spurred an increase in research and the development of innovative treatment technologies, among which those using nanoparticles receive particular interest. Among such initiatives, treatment using nanoscale zero-valent iron (nZVI) is one of the best developed. While nZVI is already well known for its site-remediation use, this perspective highlights its application in HMW treatment with metal recovery. We demonstrate several advantages of nZVI in this wastewater application, including its multifunctionality in sequestrating a wide array of metal(loid)s (> 30 species); its capability to capture and enrich metal(loid)s at low concentrations (with a removal capacity reaching 500 mg·g–1 nZVI); and its operational convenience due to its unique hydrodynamics. All these advantages are attributable to nZVI’s diminutive nanoparticle size and/or its unique iron chemistry. We also present the first engineering practice of this application, which has treated millions of cubic meters of HMW and recovered tons of valuable metals (e.g., Cu and Au). It is concluded that nZVI is a potent reagent for treating HMW and that nZVI technology provides an eco-solution to this toxic waste.

关键词： Nanoscale zero-valent iron Wastewater Heavy metal Resource recovery

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Utilization of waste vanadium-bearing resources in the preparation of rare-earth vanadate catalysts for semi-hydrogenation of ,-unsaturated aldehydes

《化学科学与工程前沿（英文）》 2022年第16卷第12期页码 1793-1806 doi: 10.1007/s11705-022-2191-x

摘要： Recycling industrial solid waste not only saves resources but also eliminates environmental concerns of toxic threats. Herein, we proposed a new strategy for the utilization of petrochemical-derived carbon black waste, a waste vanadium-bearing resource (V > 30000 ppm (10 ⁻⁶)). Chemical leaching was employed to extract metallic vanadium from the waste and the leachate containing V was used as an alternative raw material for the fabrication of vanadate nanomaterials. Through the screening of various metal cations, it was found that the contaminated Na⁺ during the leaching process showed strong competitive coordination with the vanadium ions. However, by adding foreign Ce³⁺ and Y³⁺ cations, two rare-earth vanadates, viz., flower-like CeVO₄ and spherical YVO₄ nanomaterials, were successfully synthesized. Characterization techniques such as scanning electron microscopy, transmission electron microscopy, X-ray diffraction, energy-dispersive X-ray spectroscopy, Fourier-transform infrared, and N₂ physisorption were applied to analyze the physicochemical properties of the waste-derived nanomaterials. Importantly, we found that rare-earth vanadate catalysts exhibited good activities toward the semi-hydrogenation of α,β-unsaturated aldehydes. The conversion of cinnamaldehyde and cinnamic alcohol selectivity were even higher than those of the common CeVO₄ prepared using pure chemicals (67.2% vs. 27.7% and 88.4% vs. 53.5%). Our work provides a valuable new reference for preparing vanadate catalysts by the use of abundant vanadium-bearing waste resources.

关键词： petrochemical solid wastes vanadium recovery resource utilization nanomaterials semi-hydrogenation

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End-of-life batteries management and material flow analysis in South Korea

Hyunhee Kim, Yong-Chul Jang, Yeonjung Hwang, Youngjae Ko, Hyunmyeong Yun

《环境科学与工程前沿（英文）》 2018年第12卷第3期 doi: 10.1007/s11783-018-1019-x

摘要： Consumers increasingly have worn-out batteries as electrical and electronic equipment with new technical developments are introduced into the market and quickly replace older models. As a result, large amounts of end-of-life (EOL) or waste batteries are generated. Such batteries may contain a variety of materials that includes valuable resources as well as toxic elements. Thus, the proper recycling and management of batteries is very important from the perspective of resource conservation and environmental effect. The collection and recycling of EOL batteries is relatively low in South Korea compared to other countries, although an extended producer responsibility (EPR) policy was adopted for battery recycling in 2003. In this study, the management and material flow of EOL batteries is presented to determine potential problems and quantitative flow, based on literature review, site visits to battery recycling facilities, and interviews with experts in the Korea Battery Recycling Association (KBRA), manufacturers, and regulators in government. The results show that approximately 558 tons of manganese-alkaline batteries, the largest fraction among recycling target items, was disposed in landfills or incinerators in 2015, while approximately 2,000 tons of batteries were recovered at a recycling facility by simple sorting and crushing processes. By raising environmental awareness, more diverse and effective collection systems could be established for consumers to easily dispose of EOL batteries in many places. Producers, retailers and distributors in South Korea should also play an important role in the collection of EOL batteries from consumers. Lithium-ion batteries from many electronic devices must be included in the EPR system for resource recovery.

关键词： End-of-life battery Recycling Material flow analysis (MFA) Extended producer responsibility (EPR) Resource recovery

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Water---- and nutrient and energy---- systems in urbanizing watersheds

Rodrigo VILLARROEL WALKER, Michael Bruce BECK, Jim W. HALL

《环境科学与工程前沿（英文）》 2012年第6卷第5期页码 596-611 doi: 10.1007/s11783-012-0445-4

摘要： Driven by considerations of sustainability, it has become increasingly difficult over the past 15–20 years — at least intellectually — to separate out the water infrastructure and water metabolism of cities from their intimately inter-related nutrient and energy metabolisms. Much of the focus of this difficulty settles on the wastewater component of the city’s water infrastructure and its associated fluxes of nutrients (N, P, C, and so on). Indeed, notwithstanding the massive volumes of these materials flowing into and out of the city, the notion of an urban nutrient infrastructure is conspicuous by its absence. Likewise, we do not tend to discuss, or conduct research into, “soilshed” agencies, or soilshed management, or Integrated Nutrient Resources Management (as opposed to its most familiar companion, Integrated Water Resources Management, or IWRM). The paper summarizes some of the benefits (and challenges) deriving from adopting this broader, multi-sectoral “systems” perspective on addressing water-nutrient-energy systems in city-watershed settings. Such a perspective resonates with the growing interest in broader policy circles in what is called the “water-food-energy security nexus”. The benefits and challenges of our Multi-sectoral Systems Analysis (MSA) are illustrated through computational results from two primary case studies: Atlanta, Georgia, USA; and London, UK. Since our work is part of the International Network on Cities as Forces for Good in the Environment (CFG; see www.cfgnet.org), in which other case studies are currently being initiated — for example, on Kathmandu, Nepal — we close by reflecting upon these issues of water-nutrient-energy systems in three urban settings with quite different styles and speeds of development.

关键词： cities climate change energy sector nutrient sector systems analysis resource recovery water-food-energy security

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膜技术在化工废水处理中的应用

宋伟杰,杭晓风,万印华

《中国工程科学》 2014年第16卷第12期页码 67-75

摘要：

针对化工生产过程中产生的含有多种可回收成分（多元醇、多元酸、酯类、无机盐）的废水，分别设计和开发了汽提-膜分离-精馏耦合、多级膜浓缩、渗透汽化-精馏等集成工艺。通过膜集成过程与化工生产过程的结合，可以有效地降低废水中的化学需氧量（COD），并实现废水中可回收成分的资源化利用，降低化工废水处理的综合成本，对化工产业的可持续发展具有积极意义。

关键词：膜集成技术化工废水资源化利用水回用

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温室气体提高采收率的资源化利用及地下埋存

沈平平,江怀友

《中国工程科学》 2009年第11卷第5期页码 54-59

摘要：

全球气候变化是人类迄今面临的既重大又复杂的环境问题,由于温室气体大量排放而引起的全球气候变暖问题日趋严峻，正在严重地威胁着人类赖以生存的环境，国际社会必须采取积极有效措施。2006年中国国家科技部批准国家“九七三”项目——温室气体提高石油采收率的资源化利用及地下埋存研究。建立适合中国国情的CO₂高效利用和埋存体系；实现CO₂减排的社会效益和CO₂高效利用的经济效益；发展适合中国国情的CO₂埋存地下理论、多相多组分相态理论、多相多组分非线性渗流理论和CO₂捕集与储运理论。通过上述基础研究，形成具有自主知识产权的CO₂地质埋存和高效利用的综合技术，使中国CO₂安全埋存—高效利用研究处于国际水平。必将为全球资源和环境的高水平、高效益开发和可持续发展提供理论及实践依据。

关键词：温室气体资源化利用 CO2地下埋存提高采收率

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Improved resilience measure for component recovery priority in power grids

《工程管理前沿（英文）》 2021年第8卷第4期页码 545-556 doi: 10.1007/s42524-021-0161-5

摘要： Given the complexity of power grids, the failure of any component may cause large-scale economic losses. Consequently, the quick recovery of power grids after disasters has become a new research direction. Considering the severity of power grid disasters, an improved power grid resilience measure and its corresponding importance measures are proposed. The recovery priority of failed components after a disaster is determined according to the influence of the failed components on the power grid resilience. Finally, based on the data from the 2019 Power Yearbook of each city in Shandong Province, China, the power grid resilience after a disaster is analyzed for two situations, namely, partial components failure and failure of all components. Result shows that the recovery priorities of components with different importance measures vary. The resilience evaluations under different repair conditions prove the feasibility of the proposed method.

关键词： resilience measure power grid importance measure component recovery